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The kinetics of oxidation of bis(1,4,7-triazacyclononane)nickel(II), [Ni(tacn)2]2+, by the peroxodisulphate anion has been studied in water as a function of S2O82- concentration and temperature. The reaction is first order in both the nickel(II) complex and S2O82-, with a second-order rate constant ...
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The outer-sphere oxidation of the nickel(II) complex of the deprotonated pendant-arm macrocycle, 5,5,7,12,12,14-hexamethyl-1,4,8,11-tetraazacyclotetradecane-1-acetate, [NiL1(OH2)](+) by bis-(1,4,7-triazacyclononane)nickel(III), [Ni(tacn)(2)](3+) has been studied in aqueous perchlorate media. The rea...