A nonspectroscopic method to determine the ...

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Title A nonspectroscopic method to determine the photolytic decomposition pathways of 3-chloro-3-alkyldiazirine: Carbene, diazo and rearrangement in excited state
Author(s) T. Wakahara, Y. Niino, T. Kato, Y. Maeda, T. Akasaka, Michael T. H. Liu, K. Kobayashi, S. Nagase
Journal Journal of the American Chemical Society
Date 2002
Volume 124
Issue 32
Start page 9465
End page 9468
Abstract C-60 acts as a mechanistic probe for the formation of carbene, diazo compound, and for the rearranged product via the excited state in the photolysis of 3-chloro-3-isopropyldiazirine and 3-chloro-3-chloromethyldiazirine. The carbene adds to C-60 to form methanofullerene, whereas the diazo compound adds to C-60 to form fulleroid. The olefin product arises as a result of the rearrangement in the excited state.

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